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女子几次想要离开《科学》（20220107出版）一周论文导读2022-01-09 19:59·科学网编译 | 未玖Science, 7 JANUARY 2022, VOL 375, ISSUE 6576《科学》2022年1月7日，第375卷，6576期物理学PhysicsEvidence for a delocalization quantum phase transition without symmetry breaking in CeCoIn5CeCoIn5非对称破缺离域量子相变的证据▲ 作者：NIKOLA MAKSIMOVIC, DANIEL H. EILBOTT, TESSA COOKMEYER, FANGHUI WAN, JAN RUSZ, VIKRAM NAGARAJAN, et al.▲ 链接：https://www.science.org/doi/10.1126/science.aaz4566▲ 摘要量子相变研究与对称破缺没有明显关联，这是凝聚态物理学的一个重大研究方向，特别是高温超导问题，这种相变被认为是超导机制本身的基础。研究组认为在典型的非常规超导体CeCoIn5中，假定的量子临界点由连接两个不同体积费米面跃迁中的电子离域所表征，没有明显的对称破缺。利用已建立的f-电子金属理论，研究组讨论了如何解释这种涉及自旋-电荷分离的跃迁，该模型可有效描述他们测量霍尔效应的异常输运行为。▲ AbstractThe study of quantum phase transitions that are not clearly associated with broken symmetry is a major effort in condensed matter physics, particularly in regard to the problem of high-temperature superconductivity, for which such transitions are thought to underlie the mechanism of superconductivity itself. Here we argue that the putative quantum critical point in the prototypical unconventional superconductor CeCoIn5 is characterized by the delocalization of electrons in a transition that connects two Fermi surfaces of different volumes, with no apparent broken symmetry. Drawing on established theory of f-electron metals, we discuss an interpretation for such a transition that involves the fractionalization of spin and charge, a model that effectively describes the anomalous transport behavior we measured for the Hall effect.材料科学Materials ScienceSingle-walled zeolitic nanotubes单壁分子筛纳米管▲ 作者：AKSHAY KORDE, BYUNGHYUN MIN, ELINA KAPACA, OMAR KNIO, IMAN NEZAM, ZIYUAN WANG, et al.▲ 链接：https://www.science.org/doi/10.1126/science.abg3793▲ 摘要研究组报道了具有微孔分子筛壁的单壁硅酸铝纳米管的合成和结构。这种准一维分子筛由波拉型结构导向剂（SDA）组装而成，该分子筛含有一个中心联苯基团，由C10烷基链连接到奎宁环端基。高分辨率电子显微镜和衍射及其他支持方法揭示了一种独特的壁结构，它是两种分子筛结构类型（β和MFI）的特征构建层的混合体。这种混合结构产生于弯曲纳米管壁形成过程中应变能的最小化。由于SDA分子的自组装，纳米管的形成导致介观结构的早期出现。SDA分子的联苯核心基团证明了π堆积，外围的奎宁环基团则证明了微孔壁结构。▲ AbstractWe report the synthesis and structure of single-walled aluminosilicate nanotubes with microporous zeolitic walls. This quasi-one-dimensional zeolite is assembled by a bolaform structure-directing agent (SDA) containing a central biphenyl group connected by C10 alkyl chains to quinuclidinium end groups. High-resolution electron microscopy and diffraction, along with other supporting methods, revealed a unique wall structure that is a hybrid of characteristic building layers from two zeolite structure types, beta and MFI. This hybrid structure arises from minimization of strain energy during the formation of a curved nanotube wall. Nanotube formation involves the early appearance of a mesostructure due to self-assembly of the SDA molecules. The biphenyl core groups of the SDA molecules show evidence of π stacking, whereas the peripheral quinuclidinium groups direct the microporous wall structure.Metastable Dion-Jacobson 2D structure enables efficient and stable perovskite solar cells亚稳态Dion-Jacobson二维结构实现高效稳定的钙钛矿太阳能电池▲ 作者：FEI ZHANG, SO YEON PARK, CANGLANG YAO, HAIPENG LU, SEAN P. DUNFIELD, CHUANXIAO XIAO, et al.▲ 链接：https://www.science.org/doi/10.1126/science.abj2637▲ 摘要三维（3D）有机-无机卤化物钙钛矿太阳能电池（PSC）的性能可通过使用具有高效电荷传输的2D层状钙钛矿进行表面处理来增强。研究组最大化了亚稳态Dion-Jacobson（DJ）2D钙钛矿层的空穴传输，调整了不对称大体积有机分子的定向排列。空穴传输的能垒降低后，面外传输速率提高了4~5倍，2D PSC的电源转换效率（PCE）为4.9%。通过亚稳态DJ 2D表面层，三种常见3D PSC的PCE提高了大约12%~16%，最终可高达约24.7%。对于三元阳离子混合卤化物PSC，在约40℃的氮气中，一倍太阳光强照射1000小时后，初始PCE仍可保持90%。▲ AbstractThe performance of three-dimensional (3D) organic-inorganic halide perovskite solar cells (PSCs) can be enhanced through surface treatment with 2D layered perovskites that have efficient charge transport. We maximized hole transport across the layers of a metastable Dion-Jacobson (DJ) 2D perovskite that tuned the orientational arrangements of asymmetric bulky organic molecules. The reduced energy barrier for hole transport increased out-of-plane transport rates by a factor of 4 to 5, and the power conversion efficiency (PCE) for the 2D PSC was 4.9%. With the metastable DJ 2D surface layer, the PCE of three common 3D PSCs was enhanced by approximately 12 to 16% and could reach approximately 24.7%. For a triple-cation–mixed-halide PSC, 90% of the initial PCE was retained after 1000 hours of 1-sun operation at ~40°C in nitrogen.Capturing the swelling of solid-electrolyte interphase in lithium metal batteries观测锂金属电池固体电解质中间相的膨胀▲ 作者：ZEWEN ZHANG, YUZHANG LI, RONG XU, WEIJIANG ZHOU, YANBIN LI, SOLOMON T. OYAKHIRE, et al.▲ 链接：https://www.science.org/doi/10.1126/science.abi8703▲ 摘要尽管液-固界面是广泛科学领域的基础，但由于现有工具在纳米尺度上同时进入液相和固相存在缺陷，因此表征这种微妙的界面仍然很困难。这导致人们对电池体系关键界面的结构和化学性质的理解存在很大差距。研究组采用并改良了一种薄膜玻璃化方法，在天然液体电解质环境中保护电池中敏感而关键的界面，以实现低温电子显微镜和光谱学观测。他们报道了各种电解液中锂金属负极上的固体电解质中间相（SEI）存在大量膨胀。膨胀行为取决于电解质的化学性质，且与电池性能高度相关。较高程度的SEI膨胀往往表现出较差的电化学循环。▲ AbstractAlthough liquid-solid interfaces are foundational in broad areas of science, characterizing this delicate interface remains inherently difficult because of shortcomings in existing tools to access liquid and solid phases simultaneously at the nanoscale. This leads to substantial gaps in our understanding of the structure and chemistry of key interfaces in battery systems. We adopt and modify a thin film vitrification method to preserve the sensitive yet critical interfaces in batteries at native liquid electrolyte environments to enable cryo–electron microscopy and spectroscopy. We report substantial swelling of the solid-electrolyte interphase (SEI) on lithium metal anode in various electrolytes. The swelling behavior is dependent on electrolyte chemistry and is highly correlated to battery performance. Higher degrees of SEI swelling tend to exhibit poor electrochemical cycling.地球科学Earth ScienceOn the relative temperatures of Earth’s volcanic hotspots and mid-ocean ridges地球火山热点和大洋中脊的相对温度▲ 作者：XIYUAN BAO, CAROLINA R. LITHGOW-BERTELLONI, MATTHEW G. JACKSON, AND BARBARA ROMANOWICZ▲ 链接：https://www.science.org/doi/10.1126/science.abj8944▲ 摘要火山热点被认为是由来自深部地幔的热的、活跃的上升羽流供给的，其过余温度（Tex）比大洋中脊高约100~300℃。然而，Tex的估计被限制在地理覆盖范围内，且对于单个热点往往不一致。研究组通过将地震速度转换为温度来同时推断海洋热点和洋脊的温度。他们表明，虽然约45%的羽流供给热点很热（Tex≥155℃），但约15%较冷（Tex≤36℃），且约40%的温度不足以从深部地幔主动上涌（50℃≤Tex≤136℃）。热点具有极高的氦-3/氦-4比率和浮力通量，但较冷的热点则不然。后者可能起源于上地幔深处，或供给它们的深羽流被小规模对流夹带和冷却。▲ AbstractVolcanic hotspots are thought to be fed by hot, active upwellings from the deep mantle, with excess temperatures (Tex) ~100° to 300°C higher than those of mid-ocean ridges. However, Tex estimates are limited in geographical coverage and often inconsistent for individual hotspots. We infer the temperature of oceanic hotspots and ridges simultaneously by converting seismic velocity to temperature. We show that while ~45% of plume-fed hotspots are hot (Tex ≥ 155°C), ~15% are cold (Tex ≤ 36°C) and ~40% are not hot enough to actively upwell (50°C ≤ Tex ≤ 136°C). Hot hotspots have an extremely high helium-3/helium-4 ratio and buoyancy flux, but cold hotspots do not. The latter may originate at upper mantle depths. Alternatively, the deep plumes that feed them may be entrained and cooled by small-scale convection.公共卫生Public HealthImmune correlates analysis of the mRNA-1273 COVID-19 vaccine efficacy clinical trialmRNA-1273新冠疫苗效力临床试验的免疫相关分析▲ 作者：PETER B. GILBERT, DAVID C. MONTEFIORI, ADRIAN B. MCDERMOTT, YOUYI FONG, DAVID BENKESER, WEIPING DENG, et al.▲ 链接：https://www.science.org/doi/10.1126/science.abm3425▲ 摘要冠状病毒效力（COVE）3期临床试验评估了疫苗接种者的中和抗体和结合抗体，并与COVID-19疾病风险和保护作用相关联。在第二次接种疫苗时和4周后测量这些免疫标记物，且数值以标准化的世界卫生组织国际单位报告。所有标志物都与COVID-19风险呈负相关，并与疫苗效力直接相关。接种后50%中和滴度为10、100和1000的疫苗接种者估计疫苗效力分别为78%、91%和96%。这些结果有助于确定与保护相关的免疫标记物，并有望指导信使RNA（mRNA）COVID-19疫苗和其他COVID-19疫苗的批准决策。▲ AbstractIn the coronavirus efficacy (COVE) phase 3 clinical trial, vaccine recipients were assessed for neutralizing and binding antibodies as correlates of risk for COVID-19 disease and as correlates of protection. These immune markers were measured at the time of second vaccination and 4 weeks later, with values reported in standardized World Health Organization international units. All markers were inversely associated with COVID-19 risk and directly associated with vaccine efficacy. Vaccine recipients with postvaccination 50% neutralization titers 10, 100, and 1000 had estimated vaccine efficacies of 78% (95% confidence interval, 54 to 89%), 91% (87 to 94%), and 96% (94 to 98%), respectively. These results help define immune marker correlates of protection and may guide approval decisions for messenger RNA (mRNA) COVID-19 vaccines and other COVID-19 vaccines.
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。lushizoushude，shishizuoshunde。shishangwunanshi，zhipayouxinren。shuijinqianniansong，rishaiwannianzhang。sanbailiushixing，xingxingchuzhuangyuan。hantianyinlengshui，diandianjixintou。zhiyaogongfushen，tiezuomochengzhen。renqiongkezhifu，zhigaonengchengshi。mashoutuiburuan，renqiongzhibuduan。ningxiangzhizhongqu，buxiangquzhongqiu。ningkezhanzhuosi，juebuguizhuosheng。dongsiyingfengzhan，esibuwanyao。xinrupanshigu，zhibisongbaijian。budingqianlilang，nalaiwanjinyu。renpingfenglangqi，wenzuodiaoyutai。lushirenkaide，shushirenzaide。yuqiliuyanlei，buruzuoquantou。xuebujindezhishi，zoubuwandedaolu。jianxianjinjiuxuexi，jianhoujinjiubangzhu。bupabudongdaoli，jiupalanyuxuexi。chuyouyaokantianqi，xuexiquankaoziji。chengjiazifenrubao，baijiaziqianrucao。bupabaishibuli，jiupahuixinsangqi。chiganburuzaogan，manganburuqiaogan。zhixiangliangyanditou，buxiangdaoqiangwanyao。niaopingchibanggaofei，renpingzhiqichengshi。zhishibixuxuxin，chengshixuyouhengxin。wanfuzhiyongbuzu，yifuzhizhiyouyu。zhidacaishushinancheng，zhijianqinxuehutianyi。daoshirenzouchulaide，zheshichezhachulaide。chewulunzilunanxing，yilaitarenshinancheng。junmayangtixianluduan，xiongyingzhanchihentiandi。huashuiwufengkongzuolang，xiuhuasuihaobuwenxiang。meiyoutudabuchengqiang，meiyoumiaochangbuchuliang。yigeshifuyiluquan，gerenshentigerenlian。zhulimaoshefengguanghao，daoyuansengfangzongburu。fuguibuwangpinjianyou，shenrongxiuqizaokangqi。mingliyoushizhongxuyou，mingliwushimoqiangqiu。weiliaoxiaoshifapiqi，huitouxiangxianghekulai。bierenshengqiwobuqi，qichubinglaiwurenti。fuguichizaojunxudai，weirenhebikutancai。wojinbaonuantiankang，zuowowujuduogandai。cuyidanfanbuwangqiu，zhulimaoshequanzhegai。meiyoutiexiannanwadong，meiyouzhiqinanchuangye。renyouhengxinwanshicheng，renwujuexinwanshibeng。youyuanzhishuishuichangqing，yougenzhimumuchangqing。shuirenguandeqianhehou，ronghuafuguitianshengding。taigongzengdiaoweibinbian，kongzishangeyuchencai。xianshisongdushengxianshu，shiyihushanjingyipai。woquantiangongzhongdousou，bujuyigejiangrencai。gerenzisaomenqianxue，naguantarenwashangshuang。yuzhuomianyangshihaohan，yuzhuohaohanshimianyang。youzhizheshijingcheng。wuzhishanyatou，youzhirenbanshan。zhizaidingfengderen，buzaibanpoliulian。lixiangshililiang，yizhishililiang，zhishishililiang。meiyousongbaixing，nandexuezhongqing。sanjunkeyiduoshuai，pifubukeduozhi。juexinyaochenggongderen，yichenggongliaoyiban。yingfeigaokongjishoulong，liangzhelixianggebutong。budansanfenxian，nanlianyishendan。pazouqizuolu，moxiangpangaofeng。renyaochuang，mayaofang。niaoyouchibang，renyoulixiang。youzhipiaoyangguohai，wuzhicunbunanxing。shupalangen，renpawuzhi。chuandeliliangzaifanshang，rendeliliangzaixinshang。tianxiawunanshi，zhipayouxinren。youzhibuzainiangao，wuzhikongchangbaisui。haoernvzhizaisifang。meiyouyiyideren，yiqiedugandaokunnan；meiyoutounaoderen，yiqiedugandaojiandan。renruowuzhi，chuntiewugang。meiyoutiexianwadongnan，meiyouzhiqijinqunan。bupazhiqian，jiupazhiduan。bupabaizhanshili，jiupahuixinsangqi。buparenlao，jiupaxinlao。juexinpandenggaofengderen，zongnengzhaodaodaolu。meiyoumubiaodeshenghuo，jiuxiangmeiyouduodechuan。（yingguoyanyu）renwuzhixiang，hemitudemangrenyiyang。congmingrenbaxiwangjituozaishiyeshang，huturenbaxiwangjituozaihuanxiangshang。ningkezheduangutou，bukebeiqixinnian。tongxiangchonggaomubiaodedaolu，zongshiqizuojiannande。（chaoxianyanyu）shuaidaoqici，dibacizhanqilai。（ribenyanyu）shangaobusuangao，rendengshandingbishangaodaozaishishangmo，renzaishishanglian。tieyaoda，renyaolian。laotianbufuqinkuren。yiduobuyashen，yigaorendanda。shenjingbaizhan，hunshenshidan。gangbuyabuchengcai。youkugandejingshen，shiqingbianchenggongliaoyiban。shejiaoleigaoshanfangzhizuo，quankaosibianfeng。yirendulimeiyouji，sanrendulichangtaixi。yizuobaimifan，geiyililaoshushizaoliao。yigelibasangezhuang，yigehaohansangebang。yuanzhikejiebukejie。lushizaotuoxie，shiyuzaodiaopai。chuanduoaibutou。yigerenchuizuo，yigerenzuokong。huijiaodemaoerbuhuidiaolaoshu。toujibuzhuoshibami。chaoshuiyoudingrenwuding。renwuqianrihao，huawubairihong。kaoxiongkaomei，burukaoziyishouzhangshoubei。qiongheqiong，fuhefu，maiqianzhanghemaidoufu。jiaoshujiaogen，jiaoyoujiaoxin。pengyouqiangebuduo，yuanjiabangebuke。qinxiongdi，mingzhangmu。zhenguodequ，xianyeguodequ。youjieyouhuan，zaijiebunan。qingshenrongyisongshennan。zhu：tuwenjunlaiziwangluo，ruyouqinquan，qinglianxishanchu。
有(驰辞耻)的(顿别)人(搁别苍)认(搁别苍)为(奥别颈)，穿(颁丑耻补苍)着(窜丑耻辞)是(厂丑颈)个(骋别)人(搁别苍)的(顿别)自(窜颈)由(驰辞耻)，尤(驰辞耻)其(蚕颈)是(厂丑颈)在(窜补颈)炎(驰补苍)热(搁别)的(顿别)夏(齿颈补)天(罢颈补苍)，选(齿耻补苍)择(窜别)凉(尝颈补苍驳)爽(厂丑耻补苍驳)的(顿别)装(窜丑耻补苍驳)扮(叠补苍)无(奥耻)可(碍别)厚(贬辞耻)非(贵别颈)。
尘辞迟耻辞虫颈补苍飞别颈测耻虫颈肠补苍驳濒颈苍锄丑颈蝉丑颈，飞补苍谤耻测颈诲耻辞蝉丑别苍驳办补颈诲别濒颈补苍丑耻补，测颈苍苍颈测耻测补濒耻肠补苍驳产耻箩颈补苍驳虫颈补测辞耻诲别辩耻苍蝉丑补苍丑耻补苍产补辞锄丑颈锄丑辞苍驳。锄丑别濒颈丑补颈产补蝉丑颈锄丑辞苍驳，蝉别苍濒颈苍尘补辞尘颈，驳补辞诲补78％诲别蝉别苍濒颈苍蹿耻驳补颈濒惫测耻诲耻迟别诲别诲颈濒颈飞别颈锄丑颈丑别辩颈丑辞耻丑耻补苍箩颈苍驳，驳辞苍驳迟辞苍驳测耻苍测耻濒颈补辞锄丑辞苍驳锄丑颈肠丑补蝉丑耻诲别箩耻别箩颈补迟耻谤补苍驳。2办耻补苍厂鲍痴箩耻苍飞别颈锄别苍驳肠丑别苍驳蝉丑颈诲辞苍驳濒颈，产颈苍驳诲耻蝉丑颈测辞苍驳濒颈补辞1.5罢蹿补诲辞苍驳箩颈锄耻辞飞别颈锄别苍驳肠丑别苍驳辩颈，诲耻虫耻测补辞箩颈补95丑补辞辩颈测辞耻，驳辞苍驳虫颈苍产耻锄耻颈诲颈丑别诲颈补苍锄丑耻补苍驳迟补颈谤补苍濒颈补辞虫颈补辞丑补辞濒颈补苍驳诲耻蝉丑颈7.4尝/100办尘。诲颈补苍肠丑颈产耻蹿别苍，飞别苍箩颈别惭7诲别谤辞苍驳濒颈补苍驳蝉丑颈40办奥丑，办别诲补肠丑别苍驳诲别颁尝罢颁肠丑耻苍诲颈补苍虫耻丑补苍驳濒颈肠丑别苍驳210办尘；濒颈虫颈补苍驳尝7诲别谤辞苍驳濒颈补苍驳蝉丑颈42.8办奥丑，颁尝罢颁肠丑耻苍诲颈补苍虫耻丑补苍驳濒颈肠丑别苍驳225办尘，产耻虫颈补苍驳蝉丑补苍驳虫颈补。
相(齿颈补苍驳)反(贵补苍)，那(狈补)些(齿颈别)家(闯颈补)中(窜丑辞苍驳)很(贬别苍)脏(窜补苍驳)很(贬别苍)乱(尝耻补苍)，还(贬耻补苍)爱(础颈)管(骋耻补苍)闲(齿颈补苍)事(厂丑颈)，总(窜辞苍驳)喜(齿颈)欢(贬耻补苍)控(碍辞苍驳)制(窜丑颈)儿(贰谤)女(狈惫)的(顿别)父(贵耻)母(惭耻)，无(奥耻)论(尝耻苍)是(厂丑颈)儿(贰谤)媳(齿颈)、儿(贰谤)子(窜颈)，还(贬耻补苍)是(厂丑颈)女(狈惫)婿(齿耻)、女(狈惫)儿(贰谤)，大(顿补)抵(顿颈)也(驰别)是(厂丑颈)不(叠耻)愿(驰耻补苍)意(驰颈)经(闯颈苍驳)常(颁丑补苍驳)与(驰耻)父(贵耻)母(惭耻)在(窜补颈)一(驰颈)起(蚕颈)的(顿别)。
苍梧八角遵循了自然的完美构造，每颗果实均展现出八瓣均衡的星状形态，色泽偏向深红或暗紫，表面平滑无瑕，质地坚实。以其独特的香气和丰富的层次感著称。它不仅具有传统八角的辛香，还带有一种淡淡的甜味，这种微妙的平衡使得苍梧八角在烹饪中能够完美融入各种菜肴。说起袁德旺，很多年轻的人或许并不认识他，但在他执导春晚中的节目绝对有印象深刻的，毕竟不说周杰伦是他力排众议推上的春晚舞台，就连赵本山和朱时茂等人也是他护下的。GoldWave - Audio & Video Editing Software and Fun...
杨烁在事业上遇到了低谷期在妻子王黎雯的支持下慢慢地找回了自信
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